Ultrafast Chemical Physics

The Ultrafast Chemical Physics group in the new lab

The ultrafast chemical-physics group

The main research interests in the ultrafast chemical-physics group are the study of ultrafast dynamics in the condensed phase, structure and femtosecond dynamics of proteins, and terahertz technology. One of the most interesting aspects of the work is that we cover a very broad range of sciences from the most fundamental physics to ‘dirty’ chemistry and biology. Check out ultrafast PhD projects on the departmental site. Read more about: Ultrafast spectroscopy.

About us

More information about individual group members can be found on the BCP Group Page. Go here for our picture diary. The UCP group members have ~£3M in currently running funding as primary investigators (Oct. 2009) and are part of several other projects as co-investigators.

The UCP lab

Since summer 2009, the ultrafast chemical-physics group occupies a new lab space funded in part by an S&I grant and in part by the University. It consists of a laser lab with three sections, a chemistry lab, a general lab, and a conference area. A mobile-phone movie of the lab is here (mp4, 3.7 MB).

A summary of our next paper made with Wordle

Terahertz dynamics group (KW)

One of our great interests is the ultrafast dynamics of gloopy liquid-like states of matter such as liquids, proteins, and solutions of salts and sugars. Not only are these of great practical interest (just think of ice-cream), they are difficult to study and therefore require the development of new and exciting technologies.

Molecules in the condensed phase tend to jiggle back-and-forth on a timescale of about 1 ps corresponding to a frequency of 1 THz (terahertz). Therefore, the technological arm of our research programme is all about developing technologies for terahertz spectroscopy. This ranges from (relatively) simple optical Kerr-effect experiments to the development of ultrafast terahertz-pulse sources. For those terahertz sources, the group is now using nanotechnology to convert visible light into terahertz at unprecedented efficiency.

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Ultrafast multidimensional spectroscopy group (NTH)

Our very latest work aims to observe the structural changes that occur at the active site of enzymes during their catalytic cycle. We are constructing a state-of-the-art two-dimensional infrared (2D-IR) spectrometer that will be capable of following reactions and the structure of the active site of an enzyme in real time in unprecedented detail. This 2D-IR set-up will be unique in the UK although comparable work is being done at Imperial College. The work involves collaborations with RAL (the Rutherford Appleton Labs in Oxford) and the Max Born Institute in Berlin.

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 Neil Hunt in the Ultrafast laser lab

2010 SUPA Prize studentships

The Scottish Universities Physics Alliance (SUPA) is offering up to fifteen fully funded PhD studentships for outstanding students from anywhere in the world. These prestigious and competitive awards are intended to attract outstanding students to study for a PhD in Scotland. Applicants will be registered for a PhD in physics at one of the participating Universities - such as Strathclyde. An excellent training environment will be provided by the SUPA Graduate School, giving candidates access to a wide range of courses across Scotland. The deadline for applications is 31 January 2010.

Ultrafast research group

Current members

Klaas Wynne Klaas Wynne, prof and in the department since 1996.
Neil Hunt Neil Hunt, EPSRC Advanced Research Fellow and in the department since 2004.
Robin Hochstrasser Robin Hochstrasser, visiting professor and Donner Professor of Physical Sciences at the University of Pennsylvania.
David Turton

David Turton, postdoc with KW since 2004

Spyros Kaziannis Spyros Kaziannis, postdoc with NTH since 2008.
Stefano Santabarbara Stefano Santabarbara, postdoc with NTH since January 2009.
Marco Candelaresi Marco Candelaresi, postdoc with KW since August 2009
Meenu Kumar Meenu Kumar, postdoc with NTH and Reijn Ulijn since January 2010
Scott Campbell Scott Campbell, PhD student with KW since December 2007.
Ian Stewart Ian Stewart, PhD student with NTH since September 2007.
Amy Welsh Amy Welsh, PhD student with NH since October 2008.
Rafal Kania Rafal Kania, PhD student with NTH since 2008.
Pim Frederix Pim Frederix, PhD student with NTH joint with Reijn Ulijn since March 2010.
Dacid Martin David Martin, MSci and project student with KW/DAT 2008/2009
Bob Bob Dawson, research technician
John John Revie, research technician

former members

Kitsakorn Locharoenrat

Kitsakorn LocharoenratKitsakorn received his BS in Chemical Engineering from Chulalongkorn University, Bangkok, Thailand and continued for his MS in Processing Technology at the Asian Institute of Technology, Pathumthani, Thailand. His studied for his PhD in Physical Materials Science with Prof Mizutani at the Japan Advanced Institute of Science and Technology (JAIST), Ishikawa, Japan. He was a postdoctoral researcher in the Ultrafast group in BCP in 2008/9 and worked on novel terahertz radiation emitters based on nanostructured surfaces. He now works at Research for Electronic Science in Japan.

Gregor H. Welsh

GregorGregor studied physics at Strathclyde and did his PhD in our group graduating in June 2008 on the thesis entitled "Understanding and Control of Ultrafast Currents for Terahertz Pulse Generation". Bound copies of his thesis are available in the Physics reading room and the Strathclyde library. He is currently a postdoc in the TOPS group.

 

Andy Turner

AndyAndy has been a postdoctoral fellow in the ultrafast sub-group from 2004-2006. As a theoretician, he provided theoretical insight into the varied experimental results. Andy is principally interested in using state-of-the-art computational and quantum theoretical techniques to study the dynamic properties of biological molecules. He is currently working in the Department of Chemistry at the University of Edinburgh as Research Computing Officer.

John J. Carey

John J. Carey © KWJJ studied Physics at Strathclyde and graduated with a BSc Hons in 1999. He is a former postgraduate student in KW's group and received his PhD in Physics in 2002 (You can download a copy of his thesis "Near-Field Effects of Terahertz Pulses" (PDF, 5Mb)). He has been a postdoc in the ultrafast sub-group studying varied aspects of terahertz pulses. He currently works with Coherent Scotland in Glasgow. He married Justyna (see below) and has two kids.

Gerard Giraud

Gerard GiraudGG did his undergrad partially in France and partially at Strathclyde. He was a postgrad student in our group working on optical Kerr-effect experiments to study room-temperature organic ionic liquids and proteins. His PhD thesis is online as a PDF file. GG now works at the University of Edinburgh.

 

Justyna Zawadzka

Justyna ZawadzkaJZ got her master's degree in Poland and got her PhD working in the ultrafast group as a postgrad. Her research involved making femtosecond electron pulses by using multiphoton excitation of metal surfaces and surfaces modified by nanolithography. Her PhD thesis is online as a PDF file. She married John Carey (see above) and has two kids.

 

theses

  • 12 March 2010: Our paper Universal nonexponential relaxation: Complex dynamics in simple liquids was selected JChemPhys editors’ choice as one of the most innovative and influential articles in the field of Chemical Physics in 2009. See http://jcp.aip.org/jcp/editors_choices_2009.
  • 5 January 2010: Our paper Universal nonexponential relaxation: Complex dynamics in simple liquids was the 3rd most downloaded paper of J. Chem. Phys. in December 2009.
  • 5 August 2009: Read more about our latest paper in JACS in Serving nanoparticle "soup".
  • 4 August 2009: We were joined by new postdoc Marco Candelaresi.
  • May 2009: New ultrafast chemical physics lab is ready!
  • April 2009: Find out more about 2D-IR from our recent invited Tutorial Review published in Chem Soc Rev.
  • 30/31 October 2008: The 2008 Ultrafast Chemical Physics (UCP) meeting was held at Strathclyde.
  • 14 August 2008: Neil's ERC grant featured in two press releases: Physicists in million-euro molecular movie and Three million euros boost for engineering and science research.
  • 10 July 2008: We were joined by new postdoc Kitsakorn Locharoenrat.
  • 23 May 2008: Our paper "Glasslike Behavior in Aqueous Electrolyte Solutions" was selected "Editors' Choice" in the 23 May issue of the journal Science (PDF, 800kB).
  • 12 May 2008: Groups wins £0.6M EPSRC grant "Two-dimensional terahertz–IR spectroscopy: a unique probe of ultrafast hydrogen-bond dynamics of liquid water and model systems" by KW, JOK, and DJSB.
  • 6 May 2008: Claire Neil has been awarded the Neil McDougall Bursary in Practical Oceanography by the Scottish Association for Marine Science. This is a competitively awarded scholarship which will allow her to spend 9 weeks at Dustaffnage Marine Laboratory and participate in a month-long cruise on the Royal Research Ship James Cook in the Celtic Sea. The cruise is highly relevant to her PhD work on interactions between physical mixing and optical properties in UK shelf seas.
  • 2 May 2008: Strathclyde will host the "International Workshop on Ultrafast Chemical Physics 2008 (UCP ‘08)" on 30/31 October 2008 to be held in the Senate/Court suite. Plenary speaker is Prof Robin Hochstrasser FRSE (University of Pennsylvania). Confirmed invited speakers are Prof Casey Hynes (CNRS, Paris and University of Colorado, Boulder), Prof Charles Schmuttenmaer (Yale), Prof Majed Chergui (Ecole polytechnique fédérale de Lausanne), Prof Mischa Bonn (AMOLF, Amsterdam), Prof Peter Hamm (University of Zurich), and Prof Thomas Elsaesser (Max Born Institute, Berlin). The workshop is organised by Angus J. Bain (UCL), David Klug (Imperial), Steve Meech (UEA), Neil Hunt (Strathclyde), and Klaas Wynne (Strathclyde).
  • 1 May 2008: SPRITES (Structure changes in Protein Reactions via Infrared Time Evolution Spectroscopy) a € 1M ERC Starting Grant Scheme proposal submitted by Neil Hunt has been approved for funding. The project, one of only ~300 funded projects from more than 9000 Europe-wide applications, will apply a derivative of the new ultrafast laser technique of transient 2D-IR spectroscopy to study enzymatic and protein reactions in real time.
  • 24 April 2008: Our paper "Glasslike Behavior in Aqueous Electrolyte Solutions" came out in J. Chem. Phys. A summary of the paper in simple terms (best attempt anyway) is on the page The science of syrup and traffic jams.
  • 4 March 2008: Visiting professor Robin Hochstrasser of the University of Pennsylvania has been elected Honorary Fellow of the Royal Society of Edinburgh. This is a prestigious fellowship for scientists of great international renown and we are delighted that Robin has been honoured in this way.
  • 25 June 2007: David McKee wins prestigious NERC Advanced Fellowship to study optical properties of shelf seas and other optically complex oceanic waters.
  • 18 March 2007: New paper in JACS on terahertz spectra associated with a helix to coil transition in a peptide. Read more about it in the research highlight Observing ‘The Lubricant of Life’
  • 10 January 2007: New paper on terahertz emission from nanostructured surfaces has come out in PRL. Read more about it in the research highlight nanotechnology leads to new terahertz radiation sources
  • 25 May 2006: Dr Neil Hunt has been chosen to receive an EPSRC Chemistry Advanced Research Fellowship worth about £1M. See a picture of an excited Neil in the Ultrafast picture diary.
  • March 2006: Profs David Birch and Duncan Graham and collaborators managed to secure a £5M EPSRC grant to study nanometrology.
  • January 2006: The BCP group has two new visiting professors: Prof. Robin Hochstrasser (University of Pennsylvania) and Prof. John Pickup (King's College, London)
  • November 2005: The new Wolfson Molecular Nanometrology Laboratories have been completed in the Physics and Chemistry departments. See the website of the Wolfson Nanometrology Laboratories.
  • October 2005: New ultrafast abstracts added to the ultrafast reprints section including a Kerr paper in JPCB.
  • May 2005: Dalibor Panek of the Czech Technical University is visiting the group. Dalibor's work concerns single-molecule spectroscopy of dye molecules encapsulated in porous silica.
  • March 2005: Pictures from the Optical Probes 2005 conference in Bangalore, India, are now uploaded.
  • April 2005: Integration of various sites into the BCP site; things a big mess...
  • Summer 2004: Four new people starting in the ultrafast sub-group. We got an 18-W Verdi to pump the amplifier and an FTIR. The Wolfson Nanometrology lab will be refurbished.

Also visit the web sites of the Department of Physics and the University of Strathclyde

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Open PhD and postdoctoral positions in the BCP group

Dynamics of Imidazolium Ionic Liquids from a Combined Dielectric Relaxation and Optical Kerr Effect Study: Evidence for Mesoscopic Aggregation

Chem Soc Rev review on 2D-IR

18-Mar-2010